Ultrafast spin transfer in Fe/CoO bilayers observed within 300 fs
Researchers from Freie Universität Berlin, Uppsala University and Helmholtz-Zentrum Berlin für Materialien und Energie (HZB) have directly tracked how magnetic order in a coupled Fe/CoO bilayer collapses within a few hundred femtoseconds after an ultrashort laser pulse, and identified interfacial energy transfer from Fe to CoO as the key channel for quenching the antiferromagnetic order.
The sample consists of an epitaxial 9 (±0.5) monolayer CoO film on Ag(001), capped by 9 (±1) monolayers of Fe. The CoO antiferromagnetic moments are collinear in the film plane and aligned with the Fe magnetization along an Fe ⟨100⟩ easy axis due to strong interfacial coupling; an external magnetic field can rotate this AFM spin axis by 90° in the plane via the Fe layer. Time-resolved measurements were carried out at BESSY II using 60 fs p‑polarized pump pulses at 800 or 400 nm and 100 fs polarized soft x‑ray probe pulses, providing 120 fs temporal resolution in a pump–probe reflection geometry under ultrahigh vacuum at 200 K and a 120 mT in‑plane field.
Source: https://www.spintronics-info.com/ultrafast-spin-transfer-fecoo-bilayers-observed-within-300-fs
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